High-valent iron-oxo species mediated cyclic oxidation through single-atom Fe-N6 sites with high peroxymonosulfate utilization rate

Fe singly anchored onto graphite carbon nitride (Fe-SA/PHCNS) as Fe-N6 was synthesized to realize efficient peroxymonosulfate (PMS) activation and superior organic pollutant oxidation. The Fe-N6 was the core catalytic site of activation via forming high-valent iron–oxo species (FeN6 =O) as the trans...

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Bibliographic Details
Published in:Applied catalysis. B, Environmental Environmental, 2022-05, Vol.305, p.121049, Article 121049
Main Authors: Wang, Zhiwei, Wang, Wenlong, Wang, Jin, Yuan, Yi, Wu, Qianyuan, Hu, Hongying
Format: Article
Language:English
Subjects:
Carbon
Carbon nitride
High-valent iron–oxo species
Iron
Oxidant utilization rate
Oxidation
Peroxymonosulfate activation
Pollutants
Raman spectroscopy
Single Fe atom
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