Confinement of Ultrasmall Cu/ZnOx Nanoparticles in Metal-Organic Frameworks for Selective Methanol Synthesis from Catalytic Hydrogenation of CO2

The interfaces of Cu/ZnO and Cu/ZrO2 play vital roles in the hydrogenation of CO2 to methanol by these composite catalysts. Surface structural reorganization and particle growth during catalysis deleteriously reduce these active interfaces, diminishing both catalytic activities and MeOH selectivitie...

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Bibliographic Details
Published in:Journal of the American Chemical Society 2017-03, Vol.139 (10), p.3834-3840
Main Authors: An, Bing, Zhang, Jingzheng, Cheng, Kang, Ji, Pengfei, Wang, Cheng, Lin, Wenbin
Format: Article
Language:English
Subjects:
carbon dioxide
catalysts
catalytic activity
coordination polymers
copper
hydrogenation
methanol
nanoparticles
separation
zinc oxide
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