Determining the source of unusual xenon isotopes in samples

• Published in: Journal of environmental radioactivity 2022-06, Vol.247, p.106853-106853, Article 106853
• Main Authors: Eslinger, Paul W., Ely, James, Cooper, Matthew W., Foxe, Michael, Hayes, James C., Mayer, Michael F., Panisko, Mark E., Sarathi, Ramesh
• Format: Article
• Language: English
• Subjects: Air Pollutants, Radioactive - analysis; Beta-gamma detection; Neutron activation of xenon; Radiation Monitoring - methods; Radioisotopes - analysis; Radioxenon; Radioxenon isotopes; Xenon - analysis; Xenon international system; Xenon Isotopes - analysis; Xenon Radioisotopes - analysis
• ISSN: 0265-931X; 1879-1700
• DOI: 10.1016/j.jenvrad.2022.106853

Three unusual radioactive isotopes of xenon—125Xe, 127Xe, and 129mXe—have been observed during testing of a new generation radioxenon measurement system at the manufacturing facility in Knoxville, Tennessee. These are possibly the first detections of these isotopes in environmental samples collected by automated radioxenon systems. Unfortunately, the new isotopes detected by the Xenon International sampler can interfere with quantification of the radioactive xenon isotopes used to monitor for nuclear explosions. Xenon International sampling data collected during February through September 2020 were combined with an atmospheric transport model to identify the possible release location. A source-location analyses using sample counts dominated by 125Xe strongly supports the conclusion that the release point is near (within 20 km) the sampler location. Wind patterns are not consistent with releases coming from more distant nuclear power plants. The High Flux Isotope Reactor (HFIR) and the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory are located in the region of most likely source locations. The source-location analysis cannot rule out either facility as a release location, and some of the samples may contain a combination of releases from both facilities. The source-location results using 125Xe are not unexpected because Klingberg et al. (2013) previously published the production rate of radioactive xenon isotopes from neutron activation of stable xenon in the air at the HFIR. Up to 1012 Bq of 125Xe could be produced per operational day and other xenon isotopes would be produced in lesser quantities. •A new radioxenon sampler at Knoxville, Tennessee, USA, detected 125Xe, 127Xe, and 129mXe.•These isotopes have not been previously detected in automated radioxenon samplers.•These isotopes could interfere with measurements taken for nuclear explosion monitoring.•A source-location analysis supports a release point close (20 km) to the detector.•Facilities at Oak Ridge National Laboratory are the most likely release source.