Global warming mitigation by sulphur loading in the stratosphere: dependence of required emissions on allowable residual warming rate

• Published in: Theoretical and applied climatology 2010-07, Vol.101 (1-2), p.67-81
• Main Authors: Eliseev, Alexey V., Chernokulsky, Alexandr V., Karpenko, Andrey A., Mokhov, Igor I.
• Format: Article
• Language: English
• Subjects: Aerosols; Air pollution; Air temperature; Analysis; Anthropogenic factors; Aquatic Pollution; Atmospheric carbon dioxide; Atmospheric Protection/Air Quality Control/Air Pollution; Atmospheric Sciences; Climate change; Climate change mitigation; Climate effects; Climate models; Climatology; Earth and Environmental Science; Earth Sciences; Emissions; Environmental aspects; Geoengineering; Global temperatures; Global warming; Greenhouse gases; Original Paper; Rain and rainfall; Stratosphere; Sulfates; Sulfur; Sulfur compounds; Surface temperature; Tropical environments; Waste Water Technology; Water Management; Water Pollution Control
• ISSN: 0177-798X; 1434-4483
• DOI: 10.1007/s00704-009-0198-6

An approach to mitigate global warming via sulphur loading in the stratosphere (geoengineering) is studied, employing a large ensemble of numerical experiments with the climate model of intermediate complexity IAP RAS CM. The model is forced by the historical+SRES A1B anthropogenic greenhouse gases+tropospheric sulphates scenario for 1860–2100 with additional sulphur emissions in the stratosphere in the twenty-first century. Different ensemble members are constructed by varying values of the parameters governing mass, horizontal distribution and radiative forcing of the stratospheric sulphates. It is obtained that, given a global loading of the sulphates in the stratosphere, among those studied in this paper latitudinal distributions of geoengineering aerosols, the most efficient one at the global basis is that peaked between 50° N and 70° N and with a somewhat smaller burden in the tropics. Uniform latitudinal distribution of stratospheric sulphates is a little less efficient. Sulphur emissions in the stratosphere required to stop the global temperature at the level corresponding to the mean value for 2000–2010 amount to more than 10 TgS/year in the year 2100. These emissions may be reduced if some warming is allowed to occur in the twenty-first century. For instance, if the global temperature trend S g in every decade of this century is limited not to exceed 0.10 K/decade (0.15 K/decade), geoengineering emissions of 4–14 TgS/year (2–7 TgS/year) would be sufficient. Even if the global warming is stopped, temperature changes in different regions still occur with a magnitude up to 1 K. Their horizontal pattern depends on implied latitudinal distribution of stratospheric sulphates. In addition, for the stabilised global mean surface air temperature, global precipitation decreases by about 10%. If geoengineering emissions are stopped after several decades of implementation, their climatic effect is removed within a few decades. In this period, surface air temperature may grow with a rate of several Kelvins per decade. The results obtained with the IAP RAS CM are further interpreted employing a globally averaged energy–balance climate model. With the latter model, an analytical estimate for sulphate aerosol emissions in the stratosphere required climate mitigation is obtained. It is shown that effective vertical localisation of the imposed radiative forcing is important for geoengineering efficiency.