The optimized Fenton-like activity of Fe single-atom sites by Fe atomic clusters—mediated electronic configuration modulation

The performance optimization of isolated atomically dispersed metal active sites is critical but challenging. Here, TiO₂@Fe species-N-C catalysts with Fe atomic clusters (ACs) and satellite Fe-N₄ active sites were fabricated to initiate peroxymonosulfate (PMS) oxidation reaction. The AC-induced char...

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Bibliographic Details
Published in:Proceedings of the National Academy of Sciences - PNAS 2023-04, Vol.120 (15), p.1-12, Article e2300281120
Main Authors: Mo, Fan, Song, Chunlin, Zhou, Qixing, Xue, Wendan, Ouyang, Shaohu, Wang, Qi, Hou, Zelin, Wang, Shuting, Wang, Jianling
Format: Article
Language:English
Subjects:
Active satellites
Atomic clusters
Catalysts
Configuration management
Environmental Sciences
Iron
Iron deficiency
Optimization
Oxidation
Physical Sciences
Titanium dioxide
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