The next challenge in emissions control for heavy-duty diesel vehicles: From NO x to N 2 O

• Published in: Environmental pollution (1987) 2024-11, Vol.363 (Pt 2), p.125269
• Main Authors: Chen, Hongfei, He, Liqiang, Ji, Liang, Wang, Junfang, Sun, Nannan, Zhang, Rongshuo, Wei, Yangbing, Li, Tengteng, Zhong, Xianglin, Lv, Zhihua, Zhu, Rencheng, Li, Gang
• Format: Article
• Language: English
• ISSN: 1873-6424
• DOI: 10.1016/j.envpol.2024.125269

Vehicle emissions are a major source of greenhouse gases globally. Dual selective catalytic reduction (SCR), an advanced version of single SCR, is crucial under stricter nitrogen oxide (NO ) emission standards for heavy-duty diesel vehicles (HDDVs). However, the emission characteristics of nitrous oxide (N O), a byproduct of SCR and a potent greenhouse gas, remain unclear. This study investigates the N O emissions from HDDVs equipped with single or dual SCR systems using heavy-duty chassis dynamometers under various ambient temperatures, altitudes, and loading masses. The results showed that the brake-specific emissions (EF ) of N O from HDDVs with single and dual SCRs were 76.28-269.65 mg/kWh and 147.50-170.22 mg/kWh, respectively. Notably, the dual SCR-equipped HDDV emitted 6-22 times more N O than NO under all tested conditions. As ambient temperature increased from -10 °C to 25 °C and from 25 °C to 40 °C, the average distance-based emission factors (EF ) of N O for the single SCR-equipped HDDV increased by 87.73% and 48.26%, respectively. However, the variation was not significant for the dual SCR-equipped HDDV. Under half- and full-load conditions, the average EF of N O for the single SCR-equipped HDDV increased by 47.57% and 110.92%, respectively, compared to those without loading. Similarly, N O emissions for dual SCR-equipped HDDV increased by 41.40% and 65.37% under the same loading variations. As altitude increased from 0 m to 3000 m, the average EF of N O for the single SCR-equipped HDDV decreased by 64.31%. Additionally, N O emissions were significantly affected by SCR temperature, engine power, and nitric oxide (NO)/nitrogen dioxide (NO ) ratio. These findings are crucial for setting future greenhouse gas limits of HDDVs and informing carbon reduction strategies.