Effect of grain size on gas bubble evolution in nuclear fuel: Phase-field investigations

Numerous irradiation-induced gas bubbles are created in the nuclear fuel during irradiation, leading to the change of microstructure and the degradation of mechanical and thermal properties. The grain size of fuel is one of the important factors affecting bubble evolution. In current study, we first...

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Bibliographic Details
Published in:Chinese physics B 2024-01, Vol.33 (1), p.16105-632
Main Authors: Sun, Dan, Yang, Qingfeng, Zhao, Jiajun, Gao, Shixin, Xin, Yong, Zhou, Yi, Yin, Chunyu, Chen, Ping, Zhao, Jijun, Wang, Yuanyuan
Format: Article
Language:English
Subjects:
fission gas bubble
grain size
point defects
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Summary:Numerous irradiation-induced gas bubbles are created in the nuclear fuel during irradiation, leading to the change of microstructure and the degradation of mechanical and thermal properties. The grain size of fuel is one of the important factors affecting bubble evolution. In current study, we first predict the thermodynamic behaviors of point defects as well as the interplay between vacancy and gas atom in both UO 2 and U 3 Si 2 according to ab initio approach. Then, we establish the irradiation-induced bubble phase-field model to investigate the formation and evolution of intra- and inter-granular gas bubbles. The effects of fission rate and temperature on the evolutions of bubble morphologies in UO 2 and U 3 Si 2 have been revealed. Especially, a comparison of porosities under different grain sizes is examined and analyzed. To understand the thermal conductivity as functions of grain size and porosity, the heat transfer capability of U 3 Si 2 is evaluated.
ISSN:1674-1056
2058-3834
DOI:10.1088/1674-1056/ad08a6